Rice University, in collaboration with Los Alamos National Laboratory and the Max Planck Institute, has directly observed flatband states in the kagome superconductor CsCr₃Sb₅.
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Researchers observe flatband in kagome superconductor, advancing novel materials design
Rice University researchers, in an international collaboration with colleagues at the U.S. Department of Energy's Los Alamos National Laboratory and the Max Planck Institute for Chemical Physics of Solids, have observed directly in a kagome superconductor the “flatband” energy bands that may be essential in understanding its emergent superconducting behaviors. The research, reported in the journal Nature Communications, looked at the chromium-based kagome metal CsCr₃Sb₅, which becomes a superconductor under the application of pressure. By validating theoretical predictions, the work suggests that kagome lattice geometry can lead to direct effects on the electrons, and lays the groundwork for being able to design novel superconductors, topological insulators, and spintronics elements.
As per Phys Org, Kagome metals boast a two-dimensional lattice of corner-sharing triangles; such an arrangement could harbor compact molecular orbitals — standing-wave patterns of electrons — that might, in turn, lead to unconventional superconductivity and magnetism. Flat bands in most materials are do-nothings, but in CsCr₃Sb₅, they actively mold the electronic and magnetic characteristics of the material. This finding is the experimental demonstration of the theories, which were so far known only in abstraction.
The team used advanced synchrotron techniques — angle-resolved photoemission spectroscopy (ARPES) and resonant inelastic X-ray scattering (RIXS) — to make these discoveries. ARPES mapped the emitted electrons, evidencing signatures of compact orbitals whereas RIXS measured the magnetic excitations associated with these states. These approaches jointly demonstrate that the flat bands dynamically contribute to defining the material's quantum landscape and cannot be considered as passive features.
The experimental results were also well-account for by theoretical modelling. The scientists implemented the observed features with a custom-made electronic lattice model and deduced that strong electron correlations played a crucial role. This combination of theory and experiment verified the exotic flat-band nature in CsCr₃Sb₅.
The research demonstrates the strength of interdisciplinary research in a field crossing from materials synthesis to electron and magnetic spectroscopy and theoretical physics. The work outlines a design recipe for controlling the quantum states of matter through custom tailored crystal lattice structures. The demonstration is a significant step toward utilizing kagome materials in next-generation electronics and computing, according to the Rice researchers.
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